The Guild of Calamitous Intent represents the largest organized labor force of supervillains. The Guild is the primary nemesis and antagonist for the OSI. The main article for this category is The Guild of Calamitous Intent.
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- The 5.5
- The Council of 13
- The Doom Factory
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- The Guild
- The Intangible Fancy
- The Nerve
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- The Sea Anemone
- The Sovereign
- The Splotch
- The Termite
- The Wandering Spider
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- Torrid
- Trashenstein
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- Tunnel Vision
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